Magnetic structure and ordering of multiferroic hexagonal LuFeO_{3}.

نویسندگان

  • Steven M Disseler
  • Julie A Borchers
  • Charles M Brooks
  • Julia A Mundy
  • Jarrett A Moyer
  • Daniel A Hillsberry
  • Eric L Thies
  • Dmitri A Tenne
  • John Heron
  • Megan E Holtz
  • James D Clarkson
  • Gregory M Stiehl
  • Peter Schiffer
  • David A Muller
  • Darrell G Schlom
  • William D Ratcliff
چکیده

We report on the magnetic structure and ordering of hexagonal LuFeO_{3} films of variable thickness grown by molecular-beam epitaxy on YSZ (111) and Al_{2}O_{3} (0001) substrates. These crystalline films exhibit long-range structural uniformity dominated by the polar P6_{3}cm phase, which is responsible for the paraelectric to ferroelectric transition that occurs above 1000 K. Using bulk magnetometry and neutron diffraction, we find that the system orders into a ferromagnetically canted antiferromagnetic state via a single transition below 155 K regardless of film thickness, which is substantially lower than that previously reported in hexagonal LuFeO_{3} films. The symmetry of the magnetic structure in the ferroelectric state implies that this material is a strong candidate for linear magnetoelectric coupling and control of the ferromagnetic moment directly by an electric field.

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عنوان ژورنال:
  • Physical review letters

دوره 114 21  شماره 

صفحات  -

تاریخ انتشار 2015